Biomimetic membranes made of conducting polymers doped with adenosine diphosphate (ADP)
Identifieur interne : 001F93 ( Main/Repository ); précédent : 001F92; suivant : 001F94Biomimetic membranes made of conducting polymers doped with adenosine diphosphate (ADP)
Auteurs : RBID : Pascal:13-0027628Descripteurs français
- Pascal (Inist)
- Composé biomimétique, Membrane, Polymère conducteur, Matériau dopé, ADP, Analyse chimique, Réponse transitoire, Calcium Composé, Polymérisation électrolytique, Electrode, Platine, Carbone, Etat vitreux, Microscopie électronique balayage, Spectrométrie RX dispersion énergie, Microscopie force atomique, Magnésium Composé, Potentiométrie, Electrode ITO, Etain Oxyde, Purine nucléotide, Ribonucléotide, Réaction électrochimique, Thiophène dérivé polymère, Structure surface, Morphologie, Détecteur électrochimique, Electrode optiquement transparente, Ethylènedioxythiophène polymère.
- Wicri :
English descriptors
- KwdEn :
- ADP, Atomic force microscopy, Biomimetic compound, Calcium Compounds, Carbon, Chemical analysis, Conducting polymers, Doped materials, Electrochemical detector, Electrochemical polymerization, Electrochemical reaction, Electrodes, Energy-dispersive X-ray spectrometry, Glassy state, Indium tin oxide electrode, Magnesium Compounds, Membrane, Morphology, Optically transparent electrode, Platinum, Potentiometry, Purine nucleotide, Ribonucleotide, Scanning electron microscopy, Surface structure, Thiophene derivative polymer, Tin Oxides, Transient response.
Abstract
A novel biomimetic membrane made of conducting polymer (CP) film with dispersed biological ligands (BL) is described. Adenosine diphosphate (ADP), which serves as BL, is invited as a dopant into the CP matrix formed by poly(ethylene 3,4 dioxythiophene) (PEDOT) during electropolymerization. The PEDOT-ADP films are characterized with scanning electron microscopy (SEM), energy dispersive X-ray (EDAX) and atomic force microscopy (AFM). Films are made sensitive to divalent cations (Ca2+ or Mg2+) with an optimized electrochemical oxidation and soaking processes. Resulting close-to-Nernstian potentiometric slopes are observed. Transitory potentials for the PEDOT-ADP films are studied with open-circuit measurements. Distinctively different responses for the bulk concentration changes of Ca2+ or Mg2+ ions are ascribed to a competitive ion-exchange process on the ADP sites.
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<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en" level="a">Biomimetic membranes made of conducting polymers doped with adenosine diphosphate (ADP)</title><author><name sortKey="Kupis, J" uniqKey="Kupis J">J. Kupis</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Faculty of Material Science and Ceramics, AGH - University of Science and Technology</s1><s2>30-059 Krakow</s2><s3>POL</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>Pologne</country><wicri:noRegion>30-059 Krakow</wicri:noRegion></affiliation></author><author><name sortKey="Mattinen, U" uniqKey="Mattinen U">U. Mattinen</name><affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Process Chemistry Centre, c/o Centre for Process Analytical Chemistry and Sensor Technology (ProSens), Abo Akademi University</s1><s2>20500 Turku</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>Finlande</country><wicri:noRegion>20500 Turku</wicri:noRegion></affiliation></author><author><name sortKey="Kisiel, A" uniqKey="Kisiel A">A. Kisiel</name><affiliation wicri:level="1"><inist:fA14 i1="03"><s1>Department of Chemistry, University of Warsaw</s1><s2>02-093 Warsaw</s2><s3>POL</s3><sZ>3 aut.</sZ></inist:fA14><country>Pologne</country><wicri:noRegion>02-093 Warsaw</wicri:noRegion></affiliation></author><author><name sortKey="Blaz, T" uniqKey="Blaz T">T. Blaz</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Faculty of Material Science and Ceramics, AGH - University of Science and Technology</s1><s2>30-059 Krakow</s2><s3>POL</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>Pologne</country><wicri:noRegion>30-059 Krakow</wicri:noRegion></affiliation></author><author><name sortKey="Migdalski, J" uniqKey="Migdalski J">J. Migdalski</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Faculty of Material Science and Ceramics, AGH - University of Science and Technology</s1><s2>30-059 Krakow</s2><s3>POL</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>Pologne</country><wicri:noRegion>30-059 Krakow</wicri:noRegion></affiliation></author><author><name sortKey="Lewenstam, A" uniqKey="Lewenstam A">A. Lewenstam</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Faculty of Material Science and Ceramics, AGH - University of Science and Technology</s1><s2>30-059 Krakow</s2><s3>POL</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>Pologne</country><wicri:noRegion>30-059 Krakow</wicri:noRegion></affiliation><affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Process Chemistry Centre, c/o Centre for Process Analytical Chemistry and Sensor Technology (ProSens), Abo Akademi University</s1><s2>20500 Turku</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>Finlande</country><wicri:noRegion>20500 Turku</wicri:noRegion></affiliation></author></titleStmt><publicationStmt><idno type="inist">13-0027628</idno><date when="2012">2012</date><idno type="stanalyst">PASCAL 13-0027628 INIST</idno><idno type="RBID">Pascal:13-0027628</idno><idno type="wicri:Area/Main/Corpus">001433</idno><idno type="wicri:Area/Main/Repository">001F93</idno></publicationStmt><seriesStmt><idno type="ISSN">0013-4686</idno><title level="j" type="abbreviated">Electrochim. acta</title><title level="j" type="main">Electrochimica acta</title></seriesStmt></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>ADP</term><term>Atomic force microscopy</term><term>Biomimetic compound</term><term>Calcium Compounds</term><term>Carbon</term><term>Chemical analysis</term><term>Conducting polymers</term><term>Doped materials</term><term>Electrochemical detector</term><term>Electrochemical polymerization</term><term>Electrochemical reaction</term><term>Electrodes</term><term>Energy-dispersive X-ray spectrometry</term><term>Glassy state</term><term>Indium tin oxide electrode</term><term>Magnesium Compounds</term><term>Membrane</term><term>Morphology</term><term>Optically transparent electrode</term><term>Platinum</term><term>Potentiometry</term><term>Purine nucleotide</term><term>Ribonucleotide</term><term>Scanning electron microscopy</term><term>Surface structure</term><term>Thiophene derivative polymer</term><term>Tin Oxides</term><term>Transient response</term></keywords><keywords scheme="Pascal" xml:lang="fr"><term>Composé biomimétique</term><term>Membrane</term><term>Polymère conducteur</term><term>Matériau dopé</term><term>ADP</term><term>Analyse chimique</term><term>Réponse transitoire</term><term>Calcium Composé</term><term>Polymérisation électrolytique</term><term>Electrode</term><term>Platine</term><term>Carbone</term><term>Etat vitreux</term><term>Microscopie électronique balayage</term><term>Spectrométrie RX dispersion énergie</term><term>Microscopie force atomique</term><term>Magnésium Composé</term><term>Potentiométrie</term><term>Electrode ITO</term><term>Etain Oxyde</term><term>Purine nucléotide</term><term>Ribonucléotide</term><term>Réaction électrochimique</term><term>Thiophène dérivé polymère</term><term>Structure surface</term><term>Morphologie</term><term>Détecteur électrochimique</term><term>Electrode optiquement transparente</term><term>Ethylènedioxythiophène polymère</term></keywords><keywords scheme="Wicri" type="concept" xml:lang="fr"><term>Platine</term><term>Carbone</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">A novel biomimetic membrane made of conducting polymer (CP) film with dispersed biological ligands (BL) is described. Adenosine diphosphate (ADP), which serves as BL, is invited as a dopant into the CP matrix formed by poly(ethylene 3,4 dioxythiophene) (PEDOT) during electropolymerization. The PEDOT-ADP films are characterized with scanning electron microscopy (SEM), energy dispersive X-ray (EDAX) and atomic force microscopy (AFM). Films are made sensitive to divalent cations (Ca<sup>2+</sup> or Mg<sup>2+</sup>) with an optimized electrochemical oxidation and soaking processes. Resulting close-to-Nernstian potentiometric slopes are observed. Transitory potentials for the PEDOT-ADP films are studied with open-circuit measurements. Distinctively different responses for the bulk concentration changes of Ca<sup>2+</sup> or Mg<sup>2+</sup> ions are ascribed to a competitive ion-exchange process on the ADP sites.</div></front></TEI><inist><standard h6="B"><pA><fA01 i1="01" i2="1"><s0>0013-4686</s0></fA01><fA02 i1="01"><s0>ELCAAV</s0></fA02><fA03 i2="1"><s0>Electrochim. acta</s0></fA03><fA05><s2>77</s2></fA05><fA08 i1="01" i2="1" l="ENG"><s1>Biomimetic membranes made of conducting polymers doped with adenosine diphosphate (ADP)</s1></fA08><fA11 i1="01" i2="1"><s1>KUPIS (J.)</s1></fA11><fA11 i1="02" i2="1"><s1>MATTINEN (U.)</s1></fA11><fA11 i1="03" i2="1"><s1>KISIEL (A.)</s1></fA11><fA11 i1="04" i2="1"><s1>BLAZ (T.)</s1></fA11><fA11 i1="05" i2="1"><s1>MIGDALSKI (J.)</s1></fA11><fA11 i1="06" i2="1"><s1>LEWENSTAM (A.)</s1></fA11><fA14 i1="01"><s1>Faculty of Material Science and Ceramics, AGH - University of Science and Technology</s1><s2>30-059 Krakow</s2><s3>POL</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></fA14><fA14 i1="02"><s1>Process Chemistry Centre, c/o Centre for Process Analytical Chemistry and Sensor Technology (ProSens), Abo Akademi University</s1><s2>20500 Turku</s2><s3>FIN</s3><sZ>2 aut.</sZ><sZ>6 aut.</sZ></fA14><fA14 i1="03"><s1>Department of Chemistry, University of Warsaw</s1><s2>02-093 Warsaw</s2><s3>POL</s3><sZ>3 aut.</sZ></fA14><fA20><s1>23-28</s1></fA20><fA21><s1>2012</s1></fA21><fA23 i1="01"><s0>ENG</s0></fA23><fA43 i1="01"><s1>INIST</s1><s2>1516</s2><s5>354000504041030040</s5></fA43><fA44><s0>0000</s0><s1>© 2013 INIST-CNRS. All rights reserved.</s1></fA44><fA45><s0>32 ref.</s0></fA45><fA47 i1="01" i2="1"><s0>13-0027628</s0></fA47><fA60><s1>P</s1></fA60><fA61><s0>A</s0></fA61><fA64 i1="01" i2="1"><s0>Electrochimica acta</s0></fA64><fA66 i1="01"><s0>GBR</s0></fA66><fC01 i1="01" l="ENG"><s0>A novel biomimetic membrane made of conducting polymer (CP) film with dispersed biological ligands (BL) is described. Adenosine diphosphate (ADP), which serves as BL, is invited as a dopant into the CP matrix formed by poly(ethylene 3,4 dioxythiophene) (PEDOT) during electropolymerization. The PEDOT-ADP films are characterized with scanning electron microscopy (SEM), energy dispersive X-ray (EDAX) and atomic force microscopy (AFM). Films are made sensitive to divalent cations (Ca<sup>2+</sup> or Mg<sup>2+</sup>) with an optimized electrochemical oxidation and soaking processes. Resulting close-to-Nernstian potentiometric slopes are observed. Transitory potentials for the PEDOT-ADP films are studied with open-circuit measurements. Distinctively different responses for the bulk concentration changes of Ca<sup>2+</sup> or Mg<sup>2+</sup> ions are ascribed to a competitive ion-exchange process on the ADP sites.</s0></fC01><fC02 i1="01" i2="X"><s0>001C01H02B</s0></fC02><fC02 i1="02" i2="X"><s0>001C04E</s0></fC02><fC03 i1="01" i2="X" l="FRE"><s0>Composé biomimétique</s0><s5>01</s5></fC03><fC03 i1="01" i2="X" l="ENG"><s0>Biomimetic compound</s0><s5>01</s5></fC03><fC03 i1="01" i2="X" l="SPA"><s0>Compuesto biomimético</s0><s5>01</s5></fC03><fC03 i1="02" i2="X" l="FRE"><s0>Membrane</s0><s5>02</s5></fC03><fC03 i1="02" i2="X" l="ENG"><s0>Membrane</s0><s5>02</s5></fC03><fC03 i1="02" i2="X" l="SPA"><s0>Membrana</s0><s5>02</s5></fC03><fC03 i1="03" i2="3" l="FRE"><s0>Polymère conducteur</s0><s5>03</s5></fC03><fC03 i1="03" i2="3" l="ENG"><s0>Conducting polymers</s0><s5>03</s5></fC03><fC03 i1="04" i2="3" l="FRE"><s0>Matériau dopé</s0><s5>04</s5></fC03><fC03 i1="04" i2="3" l="ENG"><s0>Doped materials</s0><s5>04</s5></fC03><fC03 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Composé</s0><s2>NC</s2><s2>NA</s2><s5>06</s5></fC07><fC07 i1="01" i2="X" l="ENG"><s0>Divalent metal Compounds</s0><s2>NC</s2><s2>NA</s2><s5>06</s5></fC07><fC07 i1="01" i2="X" l="SPA"><s0>Metal divalente Compuesto</s0><s2>NC</s2><s2>NA</s2><s5>06</s5></fC07><fN21><s1>014</s1></fN21></pA></standard></inist></record>Pour manipuler ce document sous Unix (Dilib)
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|wiki= *** parameter Area/wikiCode missing ***
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|texte= Biomimetic membranes made of conducting polymers doped with adenosine diphosphate (ADP)
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